Redesigning the Coagulation Process for Treating Water Produced from Petroleum Drilling in Water Treatment Injection Plants

Maktum Muharja; Rizki Fitria Darmayanti; Kenji Sonomoto

doi:10.33795/jtkl.v9i1.5156

Authors

Maktum Muharja Department of Chemical Engineering, Institut Teknologi Sepuluh Nopember, Kampus ITS Sukolilo, Surabaya 60111, Indonesia
Rizki Fitria Darmayanti Laboratory of Microbial Technology, Division of Systems Bioengineering, Department of Bioscience and Biotechnology, Faculty of Agriculture, Graduate School, Kyushu University, 6-10-1 Hakozaki, Higashi-ku, Fukuoka 812-8581, Japan
Kenji Sonomoto Laboratory of Microbial Technology, Division of Systems Bioengineering, Department of Bioscience and Biotechnology, Faculty of Agriculture, Graduate School, Kyushu University, 6-10-1 Hakozaki, Higashi-ku, Fukuoka 812-8581, Japan

DOI:

https://doi.org/10.33795/jtkl.v9i1.5156

Keywords:

coagulant, flocculant, oil drilling, produced water, water treatment injection plant

Abstract

This study aims to optimize the coagulation process for treating wastewater produced from petroleum drilling. The research includes redesigning the flocculator to enhance the coagulation process. The initial quality of the wastewater, characterized by parameters such as turbidity and Total Suspended Solids (TSS), did not meet the environmental quality standards stipulated by the Indonesian government. Poly Aluminum Chloride (PAC) coagulant and Polyacrylic Acid (PAA) flocculant were utilized at varying doses of 10–150 ppm and 0.25–25 ppm, respectively. The study identified the key challenges in the current coagulation and flocculation processes, including inefficiencies in pollutant removal and high operational costs. Optimal doses of 10 ppm for coagulants and 0.25 ppm for flocculants were determined, resulting in daily operational cost savings of IDR 15,865,030. The economic analysis was conducted to project the potential cost savings based on the optimized dosages, indicating a reduction in chemical costs and operational expenses. Moreover, the optimal injection distance for PAA flocculant was found to be approximately 3.5 meters from the static mixer. A new design for the flocculator was proposed, incorporating these findings to improve the overall treatment efficiency. The redesigned flocculator prototype features a 6-meter-long horizontal tube, 1.5 meters in diameter, with 15 partitions spaced 40 cm apart, and a water level difference between the inlet and outlet of around 0.67 cm. These findings suggest that coagulation redesign and optimization, along with clarifier engineering, can significantly reduce operational costs and enhance water quality for injection into the earth.

References

N. N. Ayhan, A. Aldemir, A. Özgüven, Treatment of petroleum refinery wastewater by chemical coagulation method: determination of optimum removal conditions using experimental design, Brazilian J. Chem. Eng., vol. 41, no. 1, pp. 121–137, 2024.

M. Muharja, S. Hasanah, D. A. D. Sari, M. Khoirunnafiuddin, S. N. Fadilah, R. F. Darmayanti, D. Satrio, M. Ismayati, Enhanced oil removal by graphene oxide/N,N′-methylene bisacrylamide modified magnetite-cellulose aerogel derived from ramie stem waste: Adsorption performance, kinetics, and economical analysis, Bioresour. Technol. Reports, vol. 24, pp. 101645, 2023.

O. Dkhissi, A. El Hakmaoui, M. Chatoui, R. Bouyakhsass, H. Bakraouy, T. A. Kurniawan, A. Anouzla, A. Jada, S. Souabi, Vegetable Oil Refinery Wastewater Treatment by Using the Cactus as a Bio-flocculant in the Coagulation-Flocculation Process, Water. Air. Soil Pollut., vol. 234, no. 5, pp. 1–15, 2023.

E. S. Agudosi, E. C. Abdullah, N. M. Mubarak, M. Khalid, M. Y. Pudza, N. P. Agudosi, E. D. Abutu, Pilot study of in-line continuous flocculation water treatment plant, J. Environ. Chem. Eng., vol. 6, no. 6, pp. 7185–7191, 2018.

M. Muharja, S. N. Fadilah, I. M. Arimbawa, S. Hasanah, R. F. Darmayanti, M. F. Rois, M. Asrofi, Low-cost, sustainable, and high-capacity magnetite–cellulose adsorbent from Ramie stem (Boehmeria nivea L.) as oil spill solution, Chem. Pap., vol. 76, no. 12, pp. 7429–7440, 2022.

M. S. S. Abujazar, S. U. Karaağaç, S. S. A. Amr, M. Y. D. Alazaiza, M. JK. Bashir, Recent advancement in the application of hybrid coagulants in coagulation-flocculation of wastewater : A review, J. Clean. Prod., vol. 345, pp. 131133, 2022.

B. Singh, P. Kumar, Pre-treatment of petroleum refinery wastewater by coagulation and flocculation using mixed coagulant: Optimization of process parameters using response surface methodology (RSM), J. Water Process Eng., vol. 36, pp. 101317, 2020.

Y. Sun, Y. Liu, J. Chen, Y. Huang, H. Lu, W. Yuan, Q. Yang, J. Hu, B. Yu, D. Wang, W. Xu, H. Wang, Physical pretreatment of petroleum refinery wastewater instead of chemicals addition for collaborative removal of oil and suspended solids, J. Clean. Prod., vol. 278, pp. 123821, 2021.

Z. Mumtazah, R. E. Nugraha, A. Priyangga, M. Muharja, R. F. Darmayanti, D. K. Y. Putri, H. Khotimah, Evaluating the impact of Fe2O3-Zeolite on enhancing hydrophilicity and porosity of PVDF membranes for fouling mitigation using humic acid in membrane bioreactors, Case Stud. Chem. Environ. Eng., vol. 10, pp. 100956, 2024.

R. A. Rachman, N. Widiastuti, A. S. Purnomo, A. Widjaja, Z. Mumtazah, R. F. Darmayanti, M. Muharja, Permeate flux recovery and removal foulant performances of hollow fiber polyvinylidene fluoride membrane bioreactor with peroxodisulfate activated iron (II) sulfate as a chemical cleaning agent, South African J. Chem. Eng., vol. 48, pp. 436–450, 2024.

P. E. Ovuoraye, V. I. Ugonabo, M. A. Tahir, P. A. Balogun, Kinetics-driven coagulation treatment of petroleum refinery effluent using land snail shells: An empirical approach to Environmental sustainability, Clean. Chem. Eng., vol. 4, pp. 100084, 2022.

M. Muharja, R. A. Rachman, A. Widjaja, R. F. Darmayanti, C. Wijaya, D. Satrio, Harnessing Microalgae Photobioreactors to Address Rising Sludge and Fouling Challenges in Membrane Bioreactors, ASEAN J. Chem. Eng., vol. 24, no. 2, pp. 229–241, 2024.

C. E. Santo, V. J. P. Vilar, C. M. S. Botelho, A. Bhatnagar, E. Kumar, R. A. R. Boaventura, Optimization of coagulation-flocculation and flotation parameters for the treatment of a petroleum refinery effluent from a Portuguese plant, Chem. Eng. J., vol. 183, pp. 117–123, 2012.

R. F. Darmayanti, M. Muharja, A. Widjaja, N. Widiastuti, R. A. Rachman, A. R. Widyanto, A. Halim, D. Satrio, B. Piluharto, Performance of modified hollow fiber membrane silver nanoparticles-zeolites Na–Y/PVDF composite used in membrane bioreactor for industrial wastewater treatment, Heliyon, vol. 9, no. 11, pp. e21350, 2023.

N. P. Sibiya, S. Rathilal, E. K. Tetteh, Coagulation treatment of wastewater: Kinetics and natural coagulant evaluation, Molecules, vol. 26, no. 3, pp.698, 2021.

B. Wang, Y. Shui, H. Ren, M. He, Research of combined adsorption-coagulation process in treating petroleum refinery effluent, Environ. Technol. (United Kingdom), vol. 38, no. 4, pp. 456–466, 2017.

Z. Mumtazah, R. E. Nugraha, A. Priyangga, M. Muharja, R. Fitria Darmayanti, D. K. Y. Putri, Change of Pvdf Ultrafiltration Membranes For Humus Acid Removal Applications In Water By Adding Fe2o3/Zeolite Additives, E3S Web Conf., vol. 473, pp. 03007, 2024.

B. N. Thorat, R. K. Sonwani, Current technologies and future perspectives for the treatment of complex petroleum refinery wastewater: A review, Bioresour. Technol., vol. 355, pp. 127263, 2022.

H. Ye, L. Chen, Y. Kou, Z. T. How, P. Chelme-Ayala, Q. Wang, Z. An, S. Guo, C. Chen, M. G. El-Din, Influences of coagulation pretreatment on the characteristics of crude oil electric desalting wastewaters, Chemosphere, vol. 264, pp. 128531, 2021.

A. K. Badawi, R. S. Salama, M. M. M. Mostafa, Natural-based coagulants/ flocculants as sustainable market-valued products for industrial wastewater treatment: a review of recent developments, RSC Adv., vol. 13, no. 28, pp. 19335–19355, 2023.

F. K. Katrivesis, A. D. Karela, V. G. Papadakis, C. A. Paraskeva, Revisiting of coagulation-flocculation processes in the production of potable water, J. Water Process Eng., vol. 27, pp. 193–204, 2019.

P. Bruno, R. Campo, M. G. Giustra, M. De Marchis, G. Di Bella, Bench scale continuous coagulation-flocculation of saline industrial wastewater contaminated by hydrocarbons, J. Water Process Eng., vol. 34, pp. 101156, 2020.

C. Zhao, J. Zhou, Y. Yan, L. Yang, G. Xing, H. Li, P. Wu, M. Wang, H. Zheng, Application of coagulation/ flocculation in oily wastewater treatment: A review, Sci. Total Environ., vol. 765, pp. 142795, 2021.

I. Khouni, G. Louhichi, A. Ghrabi, P. Moulin, Efficiency of a coagulation/ flocculation–membrane filtration hybrid process for the treatment of vegetable oil refinery wastewater for safe reuse and recovery, Process Saf. Environ. Prot., vol. 135, pp. 323–341, 2020.

E. K. Tetteh, S. Rathilal, Evaluation of different polymeric coagulants for the treatment of oil refinery wastewater, Cogent Eng., vol. 7, no. 1, pp. 1785756, 2020.

Y. S. Vadasarukkai, G. A. Gagnon, Influence of the Mixing Energy Consumption Affecting Coagulation and Floc Aggregation, Environ. Sci. Technol., vol. 51, no. 6, pp. 3480–3489, 2017.

S. Verma, B. Prasad, I. M. Mishra, Pretreatment of petrochemical wastewater by coagulation and flocculation and the sludge characteristics, J. Hazard. Mater., vol. 178, no. 1–3, pp. 1055–1064, 2010.

J. Ribera-Pi, M. Badia-Fabregat, D. Arias, V. Gómez, E. Taberna, J. Sanz, X. Martínez-Lladó, I. Jubany, Coagulation-flocculation and moving bed biofilm reactor as pre-treatment for water recycling in the petrochemical industry, Sci. Total Environ., vol. 715, pp. 136800, 2020.

G. Louhıchı, L. Bousselmı, A. Ghrabı, I. Khounı, Process optimization via response surface methodology in the physico-chemical treatment of vegetable oil refinery wastewater, Environ. Sci. Pollut. Res., vol. 26, no. 19, pp. 18993–19011, 2019.

A. Ghanem, T. Lemenand, D. Della Valle, H. Peerhossaini, Static mixers: Mechanisms, applications, and characterization methods – A review, Chem. Eng. Res. Des., vol. 92, no. 2, pp. 205–228, 2014.

J. P. Valdés, L. Kahouadji, O. K. Matar, Current advances in liquid–liquid mixing in static mixers: A review, Chem. Eng. Res. Des., vol. 177, pp. 694–731, 2022.

W. He, Z. Zhao, J. Nan, Z. Xie, W. Lu, The role of mixing hydrodynamics on floc growth in unbaffled square stirred-tank reactors for flocculation, J. Environ. Chem. Eng., vol. 6, no. 2, pp. 3041–3053, 2018.

K. Saxena, U. Brighu, A. Choudhary, Parameters affecting enhanced coagulation: a review, Environ. Technol. Rev., vol. 7, no. 1, pp. 156–176, 2018.

G. Rytwo, A. Rettig, Y. Gonen, Organo-sepiolite particles for efficient pretreatment of organic wastewater: Application to winery effluents, Appl. Clay Sci., vol. 51, no. 3, pp. 390–394, 2011.

Y. Chen, Y. Matsui, T. Sato, N. Shirasaki, T. Matsushita, Overlooked effect of ordinary inorganic ions on polyaluminum-chloride coagulation treatment, Water Res., vol. 235, pp. 119909, 2023.

S. Sharif, Q. uz Zaman, F. Hassan, S. Javaid, K. Arif, M. Z. Mansha, N. Ehsan, S. Nazir, R. Gul, M. Iqbal, A. Nazir, Coagulation of Metallic Pollutants from Wastewater Using a Variety of Coagulants Based on Metal Binding Interaction Studies, Zeitschrift für Physikalische Chemie, vol. 235, no. 4, pp. 467–481, 2021.

M. Ehteshami, S. Maghsoodi, E. Yaghoobnia, Optimum turbidity removal by coagulation/flocculation methods from wastewaters of natural stone processing, Desalin. Water Treat., vol. 57, no. 44, pp. 20749–20757, 2016.

S. BinAhmed, G. Ayoub, M. Al-Hindi, F. Azizi, The effect of fast mixing conditions on the coagulation–flocculation process of highly turbid suspensions using liquid bittern coagulant, Desalin. Water Treat., vol. 53, no. 12, pp. 3388–3396, 2015.

G. M. Ayoub, S. W. BinAhmed, M. Al-Hindi, F. Azizi, Coagulation of highly turbid suspensions using magnesium hydroxide: effects of slow mixing conditions., Environ. Sci. Pollut. Res. Int., vol. 21, no. 17, pp. 10502–10513, 2014.

T. J. Mohammed, E. Shakir, Effect of settling time, velocity gradient, and camp number on turbidity removal for oilfield produced water, Egypt. J. Pet., vol. 27, no. 1, pp. 31–36, 2018.

E. K. Tetteh, S. Rathilal, K. Robinson, Treatment of industrial mineral oil wastewater – effects of coagulant type and dosage, Water Pract. Technol., vol. 12, no. 1, pp. 139–145, 2017.