Innovation and Characterization of Zeolite from Matoa Fruit for Adsorption of Heavy Metals Cu(II)

Authors

  • Ainul Alim Rahman Department of Chemical Engineering, Universitas Pendidikan Muhammadiyah Sorong, Jl. KH. Ahmad Dahlan No. 1, Sorong 98457, Indonesia
  • Firmanullah Fadlil Department of Chemical Engineering, Universitas Pendidikan Muhammadiyah Sorong, Jl. KH. Ahmad Dahlan No. 1, Sorong 98457, Indonesia
  • Hajirum Tuheteru Department of Chemical Engineering, Universitas Pendidikan Muhammadiyah Sorong, Jl. KH. Ahmad Dahlan No. 1, Sorong 98457, Indonesia
  • Siti Halijah Department of Chemical Engineering, Universitas Pendidikan Muhammadiyah Sorong, Jl. KH. Ahmad Dahlan No. 1, Sorong 98457, Indonesia

DOI:

https://doi.org/10.33795/jtkl.v9i2.7390

Keywords:

adsorption, Cu metal, matoa fruit, silica, zeolite

Abstract

Matoa fruit is abundant in Papua and has not been optimally utilised. Matoa fruit consists of ash approximately 3.74%. The high ash and silica content make it highly suitable as a raw material for zeolite production. Zeolite can be used as a zeolite material to adsorb heavy metal Cu(II). Heavy metal pollution continues to increase with industrial growth. Heavy metals can harm human health. Innovation must continue addressing heavy metal pollution, such as Cu(II), to produce more efficient, cost-effective, and environmentally friendly technologies. This study aims to determine the ability of matoa fruit zeolite to adsorb heavy metal Cu(II). The characterization of zeolite was done using XRD (X-Ray Diffraction) and SEM (Scanning Electron Microscope). The synthesis process involved preparing sodium aluminate and sodium silicate solutions, followed by controlled crystallisation at 105°C for 24 hours. The zeolites were tested for adsorption with the independent variable being zeolite mass, while the dependent variables were contact time of 48 hours and stirring time of 4 hours. SEM analysis confirmed the cubic morphological characteristics of matoa fruit zeolite, classifying the product as matoa fruit zeolite. The main findings of the study showed that matoa fruit zeolite can reduce Cu metal levels in sewage-polluted water with 88.85% adsorption at 0.5 g in 50 ml of test solution.

References

A. Sinery, J. Manusawai, M. Worabay, D. Taran, E. Sirami, Palatability of Cuscus (Spilocuscus maculatus) to the Combinations of Pellet Feed Based on Organic Value, J. Sylva Lestari, vol. 12, no. 2, pp. 219–229, 2024.

Z. Mo, D. Z. Tai, H. Zhang, A. Shahab, A Comprehensive Review on the Adsorption of Heavy Metals by Zeolite Imidazole Framework (ZIF-8) Based Nanocomposite in Water, Chem. Eng. J., vol. 443, no. 5, pp. 136–320, 2022.

N. Kalakhi, Heavy metals (Zn, Cd, Cu, Pb, and Fe) assessment in sardines, Sardina pilchardus (Walbaum, 1792) from the Algerian west coast, J. Surv. Fish. Sci., vol. 10, no. 1, pp. 1–11, 2023.

J. K. Noor, A. Chamani, A. N. A. Al-Mosawy, N. Kargari, Evaluation of risk and pollution load of heavy metals (Fe, Zn, Pb, Cd, Cu, Mn, and Mo) in surface soil of Al-Qasim city, Babylon governate, Iraq, Iran. J. Heal. Environ., vol. 17, no. 3, pp. 417–440, 2024.

A. A. Rahman, F. Fadlil, H. Tuheteru, S. H. Sobabullah, Analisis Kadar Logam Tembaga (Cu) dan Besi (Fe) dalam Air Laut di Wilayah Pesisir Jembatan Puri Kota Sorong, Agitasi : Jurnal Teknik Kimia, vol. 3, no. 2, pp 1–7, 2023.

M. R. Januar, Penyisihan Logam Berat Tembaga (Cu) oleh Adsorben Mxene dengan Variasi Ukuran Partikel, pH, dan Dosis Adsorben, Undergraduate Thesis, Universitas Andalas, Padang, Indonesia, 2022.

R. Sufra, J. R. H. Panjaitan, M. Alhanif, M. Mustafa, F. Yusupandi, E. Adriansyah, G. Rahmadini, M. R. Raqin, P. Herawati, A. Suzana, Intensifikasi Pengolahan Limbah Cair Laboratorium Melalui Proses Koagulasi dan Adsorpsi Studi Pengolahan Limbah Cair Laboratorium dengan Metode Kombinasi Fisika-Kimia, J. Talenta Sipil, vol. 7, no. 1, pp. 266–275, 2024.

A. A. Rahman, M. I. Difinubun, Pengaruh pH Terhadap Kemampuan Absorben Daun Matoa Menyerap Logam Fe (III), G-Tech: Jurnal Teknologi Terapan, vol. 7, no. 3, pp. 1110–1117, 2023.

Y. Yulianis, R. Husna, N. D. I. Zulva, M. Mahidin, Adsorpsi Ion Logam Fe3+ dalam Air Asam Tambang Menggunakan Nano Zeolit Alam, Indonesia Mining Professional Journal, vol. 4, no. 1, pp. 29–38, 2022.

A. I. Abdillah, Pengaruh pH, Waktu Kontak, dan Konsentrasi pada Absorpsi Ion Logam Cd2+ Menggunakan Absorben Kitin Terikat Silang Glutaraldehid, Undergraduate Thesis, Universitas Brawijaya, Malang, Indonesia, 2014.

T. Sitanggang, A. Shofiyani, I. Syahbanu, Karakterisasi Adsorpsi Pb(II) pada Karbon Aktif dari Sabut Pinang (Areca catechu L) Teraktivasi H2SO4, Jurnal Kimia Khatulistiwa, vol. 6, no. 4, pp. 49–55, 2017.

N. Angraini, T. E. Agustina, F. Hadiah, Pengaruh pH dalam Pengolahan Air Limbah Laboratorium Dengan Metode Adsorpsi untuk Penurunan Kadar Logam Berat Pb, Cu, dan Cd, Jurnal Ilmu Lingkungan, vol. 20, no. 2, pp. 345–355, 2022.

H. Oktavianty, S. Sunardi, R. M. A. A. S. Wardani, Sintesis Zeolit dari Ekstrak Sekam Padi dan Kaleng Bekas sebagai Adsorben Penurunan Kesadahan Air, Jurnal Ilmiah Rekayasa Pertanian dan Biosistem, vol. 9, no. 2, pp. 185–192, 2021.

C. Nareswari, Pembuatan Membran PET-Pebax/Zeolit-NaY untuk Pemisahan Gas, Undergraduate Thesis, Institut Teknologi Sepuluh November, Surabaya, Indonesia, 2022.

L. M. Syawaluddin, Aktivitas Konsorsium Bakteri Pereduksi Sulfat dari Tanah Rawa dalam Pengendapan Logam Kromium (Cr) Limbah Industri Batik di Daerah Istimewa Yogyakarta, Master Thesis, Universitas Gadjah Mada, Yogjakarta, Indonesia, 2022.

N. Wang, J. Li, W. Sun, Y. Hou, L. Zhang, X. Hu, Y. Yang, X. Chen, C. Chen, B. Chen, W. Qian, Rational Design of Zinc/Zeolite Catalyst: Selective Formation of p-Xylene from Methanol to Aromatics Reaction, Angew. Chem. Int. Ed., vol. 61, no. 10, p. e202114786, 2022.

T. Nabilla, Pembuatan dan Karakterisasi Beton Polimer Menggunakan Zeolit Alam Pahae Dengan Resin Polyester Serta Serat Kulit Jagung sebagai Filler, Undergraduate Thesis, Universitas Sumatera Utara, Medan, Indonesia, 2023.

F. Fitriyah, Y. K. Krisnandi, Review : Sintesis Zeolit dari Bahan Alam dan Limbah Buangan, J. Serambi Eng., vol. 8, no. 3, pp. 6200–6207, 2023.

O. D. Anetha, Adsorben Berbahan Kulit Pisang Kepok (Musa paradisiaca, L.) untuk Pengolahan Limbah Cair Laboratorium, Undergraduate Thesis, Politeknik Negeri Lampung, Lampung, Indonesia, 2022.

G. M. Gunawan, D. Suhendar, C. D. D. Sundari, A. L. Ivansyah, S. Setiadji, Y. Rohmatulloh, Sintesis Zeolit Silikalit-1 Menggunakan Limbah Tongkol Jagung sebagai Sumber Silika, al-Kimiya, vol. 4, no. 2, pp. 91–99, 2019.

B. Salsabila, E. Nasra, H. Hardeli, I. Dewata, D. Kurniawati, Pengaruh pH dan Konsentrasi pada Penyerapan Ion Logam Cu(II) Menggunakan Kulit Buah Matoa (Pometia pinnata), Periodic, vol 12, no. 2, pp 11–15, 2023.

I. D. Fulanjari, Sintesis dan Karakterisasi Membran Nanofibers Selulosa Asetat-Zeolit untuk Adsorpsi Logam Pb (II), Undergraduate Thesis, Universitas Islam Negeri Walisongo, Semarang, Indonesia, 2022.

D. S. Asmorowati, I. I. Kristanti, S. S. Sumarti, Adsorpsi Logam Fe pada Limbah Laboratorium Kimia Menggunakan Zeolit Alam Teraktivasi Asam Sulfat, Indo. J. Chem. Sci., vol. 12, no. 1, pp. 16–21, 2023.

R. Ulandari, L. Muis, H. Suryadri, Pengaruh Waktu Terhadap Karakteristik Zeolit Sintesis Daun Bambu (Gigantochloa Atter) Menggunakan Metode Hidrotermal dan Aplikasinya Terhadap Penyerapan Ion Logam Mn2+, Jurnal Teknologi dan Inovasi Industri, vol. 5, no. 1, pp. 34–39, 2024.

E. Mohamad, I. J. Oputu, J. S. Tangio, Pemanfaatan Gulma Siam (Chromolaena Odarata L.) sebagai Adsorben Logam Timbal, Jambura J. Chem., vol. 2, no. 1, pp. 27–34, 2020.

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Published

2025-10-29